Investigation of a Citizen Above Suspicion (1970) - I watched this to better understand the climate that gave us Giallo movies not expecting to dig it, but I loved it. I think about the end of this movie all the time. Really funny and bleak and funny again.
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Another one I watched for the Cronenberg cameo and ended up loving, Nicole has some incredible looks in this movie and gives a great descent into desperation. A good double feature with Nightcrawler if you're into that.
Messiah of Evil (mostly for aesthetics)
Don't Look Now (for obvious reasons rip big don)
Lisa And The Devil (this movie became my personality for a few months, really stunning dreamlike horror)
I'd never seen The Wicker Man and didn't expect to laugh so much